- Julie Andrews Character (Mary Poppins)
- Dick Van Dyke Character (Bert/Mr. Dawes, Sr.)
- David Tomlinson Character (Mr. George W. Banks)
- Glynis Johns Character (Mrs. Winifred Banks)
- Hermione Baddeley Character (Ellen)
- Reta Shaw Character (Mrs. Brill)
- Karen Dotrice Character (Jane Banks)
- Matthew Garber Character (Michael Banks)
- Elsa Lanchester Character (Katie Nanna)
- Arthur Treacher Character (Constable Jones)
- Reginald Owen Character (Admiral Boom)
- Ed Wynn Character (Uncle Albert)
- Jane Darwell Character (The Bird Woman)
- Arthur Malet Character (Mr. Dawes Junior)
- James Logan Character (Bank Doorman)
- Don Barclay Character (Mr. Binnacle - Admiral's Servant)
- Alma Lawton Character (Mrs. Corry - Old Woman in Park)
- Marjorie Eaton Character (Miss Persimmon - Old Woman in Park)
- Marjorie Bennett Character (Miss Lark - Old Woman in Park)
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